Chemical Engineering
Mohammad Mesbah; Masumeh Jafari; Ebrahim Soroush; Shohreh Shahsavari
Abstract
Abstract In this study, a mathematical model is proposed for CO2 separation from N2/CO2 mixtureusing a hollow fiber membrane contactor by various absorbents. The contactor assumed as non-wetted membrane; radial and axial diffusions were also considered in the model development. The governing equations ...
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Abstract In this study, a mathematical model is proposed for CO2 separation from N2/CO2 mixtureusing a hollow fiber membrane contactor by various absorbents. The contactor assumed as non-wetted membrane; radial and axial diffusions were also considered in the model development. The governing equations of the model are solved via the finite element method (FEM). To ensure the accuracy of the developed model, the simulation results were validated using the reported experimental data for potassium glycinate (PG), monoethanol amine (MEA), and methyldiethanol amine (MDEA). The results of the proposed model indicated that PG absorbent has the highest removal efficiency of CO2, followed by potassium threonate (PT), MEA, amino-2-methyl-1-propanol (AMP), diethanol amine (DEA), and MDEA in sequence. In addition, the results revealed that the CO2 removal efficiency was favored by absorbent flow rate and liquid temperature, while the gas flow rate has a reverse effect. The simulation results proved that the hollow fiber membrane contactors have a good potential in the area of CO2 capture.
Ehsan Rahmandoost; Behrooz Roozbehani; Mohammad Hosein Maddahi
Abstract
CO2 emissions from combustion flue gases have turned into a major factor in global warming. Post-combustion carbon capture (PCC) from industrial utility flue gases by reactive absorption can substantially reduce the emissions of the greenhouse gas CO2. To test a new solvent (AIT600) for this purpose, ...
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CO2 emissions from combustion flue gases have turned into a major factor in global warming. Post-combustion carbon capture (PCC) from industrial utility flue gases by reactive absorption can substantially reduce the emissions of the greenhouse gas CO2. To test a new solvent (AIT600) for this purpose, a small pilot plant was used. This paper presents the results of studies on chemical methods of absorbing CO2 from flue gases with the new solvent, and evaluates the effects of operating conditions on CO2 absorption efficiency. CO2 removal rate of the AIT600 solvent was higher in comparison to the conventional monoethanolamine (MEA) solvent. The optimized temperature of the absorber column was 60 °C for CO2 absorption in this pilot plant. The overall absorption rate (Φ) and the volumetric overall mass transfer coefficient (KGaV) were also investigated.
